全文获取类型
收费全文 | 1034篇 |
免费 | 47篇 |
国内免费 | 471篇 |
专业分类
安全科学 | 61篇 |
废物处理 | 77篇 |
环保管理 | 72篇 |
综合类 | 535篇 |
基础理论 | 215篇 |
环境理论 | 1篇 |
污染及防治 | 479篇 |
评价与监测 | 54篇 |
社会与环境 | 22篇 |
灾害及防治 | 36篇 |
出版年
2023年 | 20篇 |
2022年 | 47篇 |
2021年 | 40篇 |
2020年 | 37篇 |
2019年 | 34篇 |
2018年 | 37篇 |
2017年 | 41篇 |
2016年 | 54篇 |
2015年 | 66篇 |
2014年 | 97篇 |
2013年 | 104篇 |
2012年 | 91篇 |
2011年 | 99篇 |
2010年 | 78篇 |
2009年 | 84篇 |
2008年 | 100篇 |
2007年 | 50篇 |
2006年 | 61篇 |
2005年 | 35篇 |
2004年 | 36篇 |
2003年 | 46篇 |
2002年 | 51篇 |
2001年 | 30篇 |
2000年 | 31篇 |
1999年 | 30篇 |
1998年 | 37篇 |
1997年 | 24篇 |
1996年 | 30篇 |
1995年 | 19篇 |
1994年 | 7篇 |
1993年 | 7篇 |
1992年 | 8篇 |
1991年 | 8篇 |
1990年 | 2篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1987年 | 1篇 |
1986年 | 3篇 |
1985年 | 2篇 |
1983年 | 3篇 |
排序方式: 共有1552条查询结果,搜索用时 234 毫秒
81.
伞罩型湿式脱硫除尘塔入口结构优化模拟 总被引:1,自引:1,他引:0
利用商用CFD软件Fluent,采用k-ε湍流模型和SIMPLE算法,对新型伞罩型湿式脱硫除尘塔内的三维两相流场进行数值模拟,发现了塔内烟气入口处流场所存在的不均匀性。为将其流场调节均匀从而提高脱硫除尘效率,在数值模拟的基础上提出在入口处加装直导流板、阶梯导流板和弯曲导流板,并分析塔内y=0截面速度的分布,以及z=0.21 m截面上的颗粒浓度、速度和压力等参数的分布。结果表明:通过加装阶梯导流板和弯曲导流板均可以将流场调节均匀,达到较理想状态,从而实现高效净化气体的目的。模拟结果对设备的优化设计和实际运行有一定的指导作用。 相似文献
82.
生物法同时脱硫脱硝试验研究 总被引:1,自引:0,他引:1
采用轻质陶粒生物滴滤塔处理摸拟燃煤烟气中二氧化硫和氮氧化物的试验研究,探讨生物法同时脱硫脱硝的影响因素及生物降解宏观动力学。研究结果表明,生物法能有效同时去除烟气中的二氧化硫和氮氧化物,烟气同时脱硫脱硝效率分别可达99.9%和88.9%。为获得最佳烟气同时脱硫脱硝效果,二氧化硫和氮氧化物进气负荷应分别<140 g/(m3·h)和20 g/(m3·h),循环液pH=7~8,空床停留时间为30.28 s,喷淋密度为8.81 L/(m3·h)。 相似文献
83.
以实际城市污泥为研究对象,通过采用表面活性剂作为阴极液,并考虑阴极液pH值、表面活性剂类型和电压3种因素对动电技术去除污泥中重金属(铜和镉)的影响,选用正交试验确定最佳试验条件.结果表明,采用表明活性剂作为阴极液加强动电技术去除污泥中重金属足可行的,铜和镉的去除率分别达到11.1%~52.6%和9.1%~46.7%.通过对正交试验结果进行极差和方差分析,试验的最佳条件为:电压为20 V,阴极液加入十六烷基三甲基氯化铵并控制pH值为4~6.表面活性剂的类型对动电技术去除镉具有显著影响.其中,表面活性剂类型对动电过程的影响最大,阴极液pH值次之,电压影响最小. 相似文献
84.
Atmospheric deposition of phthalate esters in a subtropical city 总被引:1,自引:0,他引:1
Feng Zeng Yujun Lin Kunyan Cui Jiaxin Wen Yongqin Ma Hongli Chen Fang Zhu Zhiling Ma Zunxiang Zeng 《Atmospheric environment (Oxford, England : 1994)》2010,44(6):834-840
In Chinese cities, air pollution has become a serious and aggravating environmental problem undermining the sustainability of urban ecosystems and the quality of urban life. Bulk atmospheric deposition samples were collected two-weekly, from February 2007 to January 2008, at three representative areas, one suburban and two urbanized, in the subtropical city, Guangzhou, China, to assess the deposition fluxes and seasonal variations of phthalate esters (PAEs). Sixteen PAE congeners in bulk deposition samples were measured and the depositional fluxes of ∑16PAEs ranged from 3.41 to 190 μg m?2 day?1, and were highly affected by local anthropogenic activities. The significant relationship between PAEs and particulate depositional fluxes (correlation coefficient R2 = 0.72, P < 0.001) showed PAEs are associated primarily with particles. Temporal flux variations of PAEs were influenced by seasonal changes in meteorological parameters, and the deposition fluxes of PAEs were obviously higher in wet season than in dry season. Diisobutyl phthalate (DiBP), Di-n-butyl phthalate (DnBP), and Di(2-ethylhexyl) phthalate (DEHP) dominated the PAE pattern in bulk depositions, which is consistent with a high consumption of the plasticizer market in China. PAE profiles in bulk deposition showed similarities exhibited in both time and space, and a weak increase of high molecular weight PAE (HMW PAE) contribution in the wet season compared to those in the dry season. Average atmospheric deposition fluxes of PAEs in the present study were significantly higher than those from other studies, reflecting strong anthropogenic inputs as a consequence of rapid industrial and urban development in the region. 相似文献
85.
Occurrence and distribution of polycyclic aromatic carbons in sludges from wastewater treatment plants in Guangdong, China 总被引:1,自引:0,他引:1
Xiangying Zeng Zheng Lin Hongyan Gui Wenlan Shao Guoying Sheng Jiamo Fu Zhiqiang Yu 《Environmental monitoring and assessment》2010,169(1-4):89-100
In this study, the occurrence and distribution of polycyclic aromatic hydrocarbons (PAHs) were investigated in six sludge samples collected from Guangdong Province, China. Concentrations of PAHs varying from 2,534.1 to 6,926.6 μg kg???1 (dry sludge) were observed in three municipal wastewater treatment plants with phenanthrene (Phe), fluoranthene, and pyrene being the main compounds. In addition, 682.6 μg kg???1 PAHs were detected in one sludge sample from a food processing plant, with fluorene, Phe, and chrysene being the main components. No PAHs were detected in sludge samples obtained from two cosmetic plants. The levels and distributional characteristics of PAHs, polychlorinated biphenyls (PCBs), and polycyclic musks (PMs) from the samples were also compared. The results of this comparison indicated that petrochemical refineries and road traffic played important roles in the PAH loads in sludge, while PMs primarily originated from domestic wastewater and industrial wastewater from cosmetic plants. Finally, the presence of 98.8 μg kg???1 PCBs in sludge suggested diffusional emission sources from electrical components containing PCBs. 相似文献
86.
Mianzhi Wang Yongxue Sun Peng Liu Jing Sun Qin Zhou Wenguang Xiong Zhenling Zeng 《Environmental science and pollution research international》2017,24(26):20949-20958
This study aimed to determine the occurrence, abundance, and fate of nine important antimicrobial resistance genes (ARGs) (sul1, sul2, tetB, tetM, ermB, ermF, fexA, cfr, and Intl1) in the simulated soil and pond microcosms following poultry and swine manure application. Absolute quantitative PCR method was used to determine the gene copies. The results were modeled as a logarithmic regression (N?=?mlnt?+?b) to explore the fate of target genes. Genes sul1, Intl1, sul2, and tetM had the highest abundance following the application of the two manure types. The logarithmic regression model fitted the results well (R 2 values up to 0.99). The reduction rate of all genes (except for the genes fexA and cfr) in manure-pond microcosms was faster than those in manure-soil microcosms. Importantly, sul1, intl1, sul2, and tetM had the lowest reduction rates in all the samples and the low reduction rates of tetM was the first time to be reported. These results indicated that ARG management should focus on using technologies for the ARG elimination before the manure applications rather than waiting for subsequent attenuation in soil or water, particularly the ARGs (such as sul1, intl1, sul2, and tetM investigated in this study) that had high abundance and low reduction rate in the soil and water after application of manure. 相似文献
87.
Lan Q Cui K Zeng F Zhu F Liu H Chen H Ma Y Wen J Luan T Sun G Zeng Z 《Environmental monitoring and assessment》2012,184(8):4921-4929
Phthalate esters (PAEs) were examined in indoor and outdoor dust samples from the subtropical city of Guangzhou, China. The ∑(16)PAEs concentrations ranged from 121 to 3,223 μg g(-1) dust, with the median concentration of 840 μg g(-1) dust. Significantly higher concentrations of PAEs in dust samples were found in offices where electrical and electronic devices, carpet pads, and office furniture were widely used. Of the 16 PAEs, diisobutyl phthalate (DiBP), di-n-butyl phthalate (DnBP), and di(2-ethylhexyl) phthalate (DEHP) dominated the PAEs in indoor and outdoor dust samples, and accounted for >96.8% and >93.1% of the ∑(16)PAEs concentrations, respectively. The median daily inhalation exposure of ∑(16)PAEs were 3.53 and 0.247 μg kg(-1) body weight day(-1), and at the 95(th) percentile were 7.62 and 0.530 μg kg(-1) body weight day(-1), up on the measured concentrations and estimated dust ingestion rates, respectively, for toddles and adults. The ubiquitous distribution of PAEs as noted in this study suggests the need for detailed assessment of PAEs concentrations using more sites and to further investigate the factors influencing PAEs exposure in China. 相似文献
88.
Wenying Chen Yves-Michel Le Nindre Ruina Xu Delphine Allier Fei Teng Kim Domptail Xing Xiang Laura Guillon Jiyong Chen Lingyan Huang Rongshu Zeng 《International Journal of Greenhouse Gas Control》2010,4(2):341-350
A method, based on spatial analysis of the different criteria to be taken into consideration for building scenarios of CO2 capture and storage (CCS), has been developed and applied to real case studies in the Hebei province. Totally 88 point sources (42 from power sector, 9 from iron and steel, 18 from cement, 16 from ammonia, and 3 from oil refinery) are estimated and their total emission amounts to 231.7 MtCO2/year with power, iron and steel, cement, ammonia and oil refinery sharing 59.13%, 25.03%, 11.44%, 3.5%, and 0.91%, respectively. Storage opportunities can be found in Hebei province, characterised by a strong tectonic subsidence during the Tertiary, with several kilometres of accumulated clastic sediments. Carbon storage potential for 25 hydrocarbon fields selected from the Huabei complex is estimated as 215 MtCO2 with optimistic assumption that all recovered hydrocarbon could be replaced by an equivalent volume of CO2 at reservoir conditions. Storage potential for aquifers in the Miocene Guantao formation is estimated as 747 MtCO2 if closed aquifer assumed or 371 MtCO2 if open aquifer and single highly permeable horizon assumed. Due to poor knowledge on deep hydrogeology and to pressure increase in aquifer, injecting very high rates requested by the major CO2 sources (>10 MtCO2/year) is the main challenge, therefore piezometry and discharge must be carefully controlled. A source sink matching model using ArcGIS software is designed to find the least-cost pathway and to estimate transport route and cost accounting for the additional costs of pipeline construction due to landform and land use. Source sink matching results show that only 15–25% of the emissions estimated for the 88 sources can be sequestrated into the hydrocarbon fields and the aquifers if assuming sinks should be able to accommodate at least 15 years of the emissions of a given source. 相似文献
89.
90.
In order to measure groundwater age and design nuclear waste disposal sites, it is important to understand the sorption behavior of tritium on soils. In this study, batch tests were carried out using four soils from China: silty clays from An County and Jiangyou County in Sichuan Province, both of which could be considered candidate sites for Very Low Level Waste disposal; silty sand from Beijing; and loess from Yuci County in Shanxi Province, a typical Chinese loess region. The experimental results indicated that in these soil media, the distribution coefficient of tritium is slightly influenced by adsorption time, water/solid ratio, initial tritium specific activity, pH, and the content of humic and fulvic acids. The average distribution coefficient from all of these influencing factors was about 0.1-0.2 mL/g for the four types of soil samples. This relatively modest sorption of tritium in soils needs to be considered in fate and transport studies of tritium in the environment. 相似文献